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- W3102603062 abstract "Quantum light sources in solid-state systems are of major interest as a basic ingredient for integrated quantum photonic technologies. The ability to tailor quantum emitters via site-selective defect engineering is essential for realizing scalable architectures. However, a major difficulty is that defects need to be controllably positioned within the material. Here, we overcome this challenge by controllably irradiating monolayer MoS2 using a sub-nm focused helium ion beam to deterministically create defects. Subsequent encapsulation of the ion exposed MoS2 flake with high-quality hBN reveals spectrally narrow emission lines that produce photons in the visible spectral range. Based on ab-initio calculations we interpret these emission lines as stemming from the recombination of highly localized electron-hole complexes at defect states generated by the local helium ion exposure. Our approach to deterministically write optically active defect states in a single transition metal dichalcogenide layer provides a platform for realizing exotic many-body systems, including coupled single-photon sources and interacting exciton lattices that may allow the exploration of Hubbard physics." @default.
- W3102603062 created "2020-11-23" @default.
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- W3102603062 date "2019-06-21" @default.
- W3102603062 modified "2023-10-17" @default.
- W3102603062 title "Site-selectively generated photon emitters in monolayer MoS2 via local helium ion irradiation" @default.
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- W3102603062 doi "https://doi.org/10.1038/s41467-019-10632-z" @default.
- W3102603062 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/6588625" @default.
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