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• W3102666734 abstract "We perform time-resolved ionization spectroscopy measurements of the excited state dynamics of CH2I2 and CH2IBr following photoexcitation in the deep UV. The fragment ions produced by ionization with a vacuum-ultraviolet probe pulse are measured with velocity map imaging, and the momentum resolved yields are compared with trajectory surface hopping calculations of the measurement observable. Together with recent time-resolved photoelectron spectroscopy measurements of the same dynamics, these results provide a detailed picture of the coupled electronic and nuclear dynamics involved. Our measurements highlight the non-adiabatic coupling between electronic states, which leads to notable differences in the dissociation dynamics for the two molecules." @default.
• W3102666734 created "2020-11-23" @default.
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• W3102666734 date "2020-11-10" @default.
• W3102666734 modified "2023-10-17" @default.
• W3102666734 title "Excited-state dynamics of CH₂I₂ and CH₂IBr studied with UV-pump VUV-probe momentum-resolved photoion spectroscopy" @default.
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• W3102666734 doi "https://doi.org/10.1063/5.0026177" @default.
• W3102666734 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33187419" @default.
• W3102666734 hasPublicationYear "2020" @default.
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