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- W3102912106 abstract "Using computer simulations we investigate the homogeneous crystal nucleation in suspensions of colloidal hard dumbbells. The free energy barriers are determined by Monte Carlo simulations using the umbrella sampling technique. We calculate the nucleation rates for the plastic crystal and the aperiodic crystal phase using the kinetic prefactor as determined from event driven molecular dynamics simulations. We find good agreement with the nucleation rates determined from spontaneous nucleation events observed in event driven molecular dynamics simulations within error bars of one order of magnitude. We study the effect of aspect ratio of the dumbbells on the nucleation of plastic and aperiodic crystal phases and we also determine the structure of the critical nuclei. Moreover, we find that the nucleation of the aligned CP1 crystal phase is strongly suppressed by a high free energy barrier at low supersaturations and slow dynamics at high supersaturations." @default.
- W3102912106 created "2020-11-23" @default.
- W3102912106 creator A5030640930 @default.
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- W3102912106 date "2011-01-18" @default.
- W3102912106 modified "2023-10-09" @default.
- W3102912106 title "Crystal nucleation of colloidal hard dumbbells" @default.
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- W3102912106 doi "https://doi.org/10.1063/1.3528222" @default.
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