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• W3102921105 startingPage "094705" @default.
• W3102921105 abstract "We provide a prescription to construct a microscopic model for heavy lanthanide systems such as Yb and Tm compounds by exploiting a j – j coupling scheme. Here we consider a situation with a large spin–orbit coupling, in which j =5/2 sextet is fully occupied, while j =7/2 octet is partially occupied, where j denotes total angular momentum. We evaluate crystalline electric field potentials and Coulomb interactions among the states of the j =7/2 octet to construct a local Hamiltonian in the j – j coupling scheme. Then, it is found that the local f -electron states composed of the j =7/2 octet agree quite well with those of seven f orbitals even for a realistic value of the spin–orbit coupling. As an example of the application of the present model, we discuss low-temperature multipole states of Yb- and Tm-based filled skutterudites by analyzing multipole susceptibility of the Anderson model in the j – j coupling scheme with the use of a numerical renormalization group technique. From the comparison with the numerical results of the seven-orbital Anderson model, it is concluded that the multipole state is also well reproduced by the j – j coupling model, even when we include the hybridization between conduction and f electrons for the realistic value of the spin–orbit coupling. Finally, we briefly discuss future applications of the present prescription for theoretical research on heavy lanthanide compounds." @default.
• W3102921105 created "2020-11-23" @default.
• W3102921105 creator A5086622241 @default.
• W3102921105 date "2010-09-15" @default.
• W3102921105 modified "2023-09-23" @default.
• W3102921105 title "Construction of a Microscopic Model for Yb and Tm Compounds on the Basis of a<b>j</b>–<b>j</b>Coupling Scheme" @default.
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• W3102921105 doi "https://doi.org/10.1143/jpsj.79.094705" @default.
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