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- W3103003374 abstract "We studied the crystal structure and spin state of MnP under high pressure with synchrotron x-ray diffraction and x-ray emission spectroscopy (XES). MnP has an exceedingly strong anisotropy in compressibility, with the primary compressible direction along the b axis of the Pnma structure. XES reveals a pressure-driven quenching of the spin state in MnP. First-principles calculations suggest that the strongly anisotropic compression behavior significantly enhances the dispersion of the Mn d-orbitals and the splitting of the d-orbital levels compared to the hypothetical isotropic compression behavior. Thus, we propose spin quenching results mainly from the significant enhancement of the itinerancy of d electrons and partly from spin rearrangement occurring in the split d-orbital levels near the Fermi level. This explains the fast suppression of magnetic ordering in MnP under high pressure. The spin quenching lags behind the occurrence of superconductivity at ∼8 GPa implying that spin fluctuations govern the electron pairing for superconductivity." @default.
- W3103003374 created "2020-11-23" @default.
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- W3103003374 date "2018-02-05" @default.
- W3103003374 modified "2023-10-13" @default.
- W3103003374 title "Spin quenching assisted by a strongly anisotropic compression behavior in MnP" @default.
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- W3103003374 doi "https://doi.org/10.1088/1367-2630/aaa3c3" @default.
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