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• W3103027098 abstract "In a cluster crystal, each lattice site is occupied by multiple soft-core particles. As the number density is increased at zero temperature, a `cascade' of isostructural phase transitions can occur between states whose site occupancy differs by unity. For low but finite temperature, each of these transitions terminates in a critical point. Using tailored Monte Carlo simulation techniques we have studied such demixing cascades in systems of soft particles interacting via potentials of the generalized exponential form $u(r)=epsilonexp[-(r/sigma)^n]$. We have estimated the critical parameters of the first few transitions in the cascade as a function of the softness parameter $n$. The critical temperature and pressure exhibit non-monotonic behaviour as $n$ is varied, although the critical chemical potential remains monotonic. The trends for the pressure and chemical potential are confirmed by cell model calculations at zero temperature. As $nto 2^+$, all the transitions that we have observed are preempted by melting although we cannot rule out that clustering transitions survive at high density." @default.
• W3103027098 created "2020-11-23" @default.
• W3103027098 creator A5036123293 @default.
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• W3103027098 date "2014-09-04" @default.
• W3103027098 modified "2023-10-17" @default.
• W3103027098 title "Demixing cascades in cluster crystals" @default.
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• W3103027098 doi "https://doi.org/10.1063/1.4894374" @default.
• W3103027098 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/25194390" @default.
• W3103027098 hasPublicationYear "2014" @default.
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