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- W3103296032 abstract "Abstract An aminocatalytic privileged diversity‐oriented synthesis (ApDOS) strategy utilizing trienamine catalysis for the construction of diverse and complex thiopyrans‐piperidone fused rings through a thia‐Diels–Alder/nucleophilic ring‐closing sequence by using dithioamides as activated heterodienophiles is reported. Following this strategy, a super cascade reaction to assemble nine fused rings can be achieved by employing a bis‐dithioamide. Additionally, by linking an indole moiety on the dithioamide, a Pictet–Spengler type reaction can be promoted once the cascade sequence has been achieved, leading to more complex penta‐ hexa‐ and heptacyclic fused ring derivatives in a one‐pot process. This investigation opens new perspectives for the synthesis of a new class of complex and diverse thiopyrans that contribute to populate new relevant regions in the chemical space." @default.
- W3103296032 created "2020-11-23" @default.
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- W3103296032 date "2020-12-09" @default.
- W3103296032 modified "2023-10-18" @default.
- W3103296032 title "Organocatalytic Cascade Reactions for the Diversification of Thiopyrano‐Piperidone Fused Rings Utilizing Trienamine Activation" @default.
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- W3103296032 doi "https://doi.org/10.1002/chem.202004553" @default.
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