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- W3103313691 abstract "Understanding over-limiting current (faster than diffusion) is a long-standing challenge in electrochemistry with applications in desalination and energy storage. Known mechanisms involve either chemical or hydrodynamic instabilities in unconfined electrolytes. Here, it is shown that over-limiting current can be sustained by surface conduction in nanopores, without any such instabilities and used to control dendritic growth during electrodeposition. Copper electrodeposits are grown in anodized aluminum oxide membranes with polyelectrolyte coatings to modify the surface charge. At low currents, uniform electroplating occurs, unaffected by surface modification due to thin electric double layers, but the morphology changes dramatically above the limiting current. With negative surface charge, growth is enhanced along the nanopore surfaces, forming surface dendrites and nanotubes behind a deionization shock. With positive surface charge, dendrites avoid the surfaces and are either guided along the nanopore centers or blocked from penetrating the membrane." @default.
- W3103313691 created "2020-11-23" @default.
- W3103313691 creator A5020245973 @default.
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- W3103313691 creator A5040301944 @default.
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- W3103313691 date "2014-11-14" @default.
- W3103313691 modified "2023-10-16" @default.
- W3103313691 title "Over-limiting Current and Control of Dendritic Growth by Surface Conduction in Nanopores" @default.
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- W3103313691 doi "https://doi.org/10.1038/srep07056" @default.
- W3103313691 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/4231330" @default.
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