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- W3103403708 abstract "The surface of poly (p-phenylene benzobisoxazole) (PBO) fibers with self-healing and ultraviolet (UV)-resistance performance play the key role in prolonging their service lifespan. Although great advances have been made in the single aspect of above two properties, integration of self-healing and anti-UV performance into the surface of PBO fiber is still a challenge. In this study, the coagulation strategy mediated by metal-organic framework (MOF) is proposed to construct the multifunctional surface of PBO fibers. The spindle-like iron (III)-based MOF (MIL-88B-NH2) nanocrystals are firstly immobilized onto the surface of PBO-COOH through hydrothermal reaction, then serving as the medium layer to further immobilize sufficient graphene oxide (GO) nanosheets. Benefitting from the favorable near-infrared (NIR, 808 nm) photothermal conversion performance of GO nanolayers, the monofilament [email protected]2-GO-TPU (thermoplastic polyurethane) exhibited a stable and high self-healing efficiency (approximately 80%) within five cycle times. Meanwhile, the cooperative adsorption and shielding weaken effects of MOF-GO nanolayers enabled PBO fibers with excellent anti-UV properties that are superior to much reported literatures after 96 h aging time and eventually increased by 75% compared with untreated PBO fiber. In view of the varieties and multifunctionalities of MOFs and carbon nanomaterials, MOF-mediated coagulation strategy would provide guidance for preparing multifunctional composite materials." @default.
- W3103403708 created "2020-11-23" @default.
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- W3103403708 date "2021-04-01" @default.
- W3103403708 modified "2023-10-15" @default.
- W3103403708 title "Facile immobilization of graphene nanosheets onto PBO fibers via MOF-mediated coagulation strategy: Multifunctional interface with self-healing and ultraviolet-resistance performance" @default.
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- W3103403708 doi "https://doi.org/10.1016/j.jcis.2020.11.026" @default.
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