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• W3105585217 abstract "Water inside the low-dimensional carbon structures has been considered seriously owing to fundamental interest in its flow and structures as well as its practical impact. Recently, the anomalous perfect penetration of water through graphene oxide membrane was demonstrated although the membrane was impenetrable for other liquids and even gases. The unusual auxetic behavior of graphene oxide in the presence of water was also reported. Here, on the basis of first-principles calculations, we establish atomistic models for hybrid systems composed of water and graphene oxides revealing the anomalous water behavior inside the stacked graphene oxides. We show that formation of hexagonal ice bilayer in between the flakes as well as melting transition of ice at the edges of flakes are crucial to realize the perfect water permeation across the whole stacked structures. The distance between adjacent layers that can be controlled either by oxygen reduction process or pressure is shown to determine the water flow thus highlighting a unique water dynamics in randomly connected two-dimensional spaces." @default.
• W3105585217 created "2020-11-23" @default.
• W3105585217 creator A5014915178 @default.
• W3105585217 creator A5052554493 @default.
• W3105585217 creator A5089610449 @default.
• W3105585217 date "2013-07-19" @default.
• W3105585217 modified "2023-09-30" @default.
• W3105585217 title "Origin of Anomalous Water Permeation through Graphene Oxide Membrane" @default.
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• W3105585217 doi "https://doi.org/10.1021/nl4020292" @default.
• W3105585217 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/23859009" @default.
• W3105585217 hasPublicationYear "2013" @default.
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