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• W3105608765 abstract "Barlowite, Cu$_{4}$(OH)$_{6}$FBr, has attracted much attention as the parent compound of a new series of quantum spin liquid candidates, Zn$_{x}$Cu$_{4-x}$(OH)$_{6}$FBr. While it is known to undergo a magnetic phase transition to a long-range ordered state at $T_{N} = 15$ K, there is still no consensus over either its nuclear or magnetic structures. Here, we use comprehensive powder neutron diffraction studies on deuterated samples of barlowite to demonstrate that the only space group consistent with the observed nuclear and magnetic diffraction at low-temperatures is the orthorhombic $Pnma$ space group. We furthermore conclude that the magnetic intensity at $T < T_{N}$ is correctly described by the $Pn^prime m^prime a$ magnetic space group, which crucially allows the ferromagnetic component observed in previous single-crystal and powder magnetisation measurements. As such, the magnetic structure of barlowite resembles that of the related material clinoatacamite, Cu$_{4}$(OH)$_{6}$Cl$_{2}$, the parent compound of the well-known quantum spin liquid candidate hebertsmithite, ZnCu$_{3}$(OH)$_{6}$Cl$_{2}$." @default.
• W3105608765 created "2020-11-23" @default.
• W3105608765 creator A5039310870 @default.
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• W3105608765 date "2018-11-27" @default.
• W3105608765 modified "2023-09-27" @default.
• W3105608765 title "Nuclear and magnetic structures of the frustrated quantum antiferromagnet barlowite,<mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:mrow><mml:msub><mml:mi>Cu</mml:mi><mml:mn>4</mml:mn></mml:msub><mml:msub><mml:mrow><mml:mo>(</mml:mo><mml:mi>OH</mml:mi><mml:mo>)</mml:mo></mml:mrow><mml:mn>6</mml:mn></mml:msub><mml:mi>FBr</mml:mi></mml:mrow></mml:math>" @default.
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• W3105608765 doi "https://doi.org/10.1103/physrevmaterials.2.111405" @default.
• W3105608765 hasPublicationYear "2018" @default.
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