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- W3106239908 abstract "We investigate how correlated fluctuations affect oscillatory features in rephasing and non-rephasing two-dimensional (2D) electronic spectra of a model dimer system. Based on a beating map analysis, we show that non-secular environmental couplings induced by uncorrelated fluctuations lead to oscillations centered at both cross- and diagonal-peaks in rephasing spectra as well as in non-rephasing spectra. Using an analytical approach, we provide a quantitative description of the non-secular effects in terms of the Feynman diagrams and show that the environment-induced mixing of different inter-excitonic coherences leads to oscillations in the rephasing diagonal-peaks and non-rephasing cross-peaks. We demonstrate that as correlations in the noise increase, the lifetime of oscillatory 2D signals is enhanced at rephasing cross-peaks and non-rephasing diagonal-peaks, while the other non-secular oscillatory signals are suppressed. We discuss that the asymmetry of 2D lineshapes in the beating map provides information on the degree of correlations in environmental fluctuations. Finally we investigate how the oscillatory features in 2D spectra are affected by inhomogeneous broadening." @default.
- W3106239908 created "2020-11-23" @default.
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- W3106239908 date "2017-01-13" @default.
- W3106239908 modified "2023-09-27" @default.
- W3106239908 title "Signatures of spatially correlated noise and non-secular effects in two-dimensional electronic spectroscopy" @default.
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- W3106239908 cites W1975391438 @default.
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- W3106239908 cites W1977436968 @default.
- W3106239908 cites W1977832464 @default.
- W3106239908 cites W1980799223 @default.
- W3106239908 cites W1981417082 @default.
- W3106239908 cites W1981627037 @default.
- W3106239908 cites W1982972906 @default.
- W3106239908 cites W1989513865 @default.
- W3106239908 cites W1989833306 @default.
- W3106239908 cites W1993965665 @default.
- W3106239908 cites W2007593774 @default.
- W3106239908 cites W2009688314 @default.
- W3106239908 cites W2009730628 @default.
- W3106239908 cites W2011298104 @default.
- W3106239908 cites W2014592731 @default.
- W3106239908 cites W2015609257 @default.
- W3106239908 cites W2017964195 @default.
- W3106239908 cites W2020125662 @default.
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- W3106239908 cites W2044111627 @default.
- W3106239908 cites W2044133255 @default.
- W3106239908 cites W2044950323 @default.
- W3106239908 cites W2045192660 @default.
- W3106239908 cites W2049160245 @default.
- W3106239908 cites W2049846301 @default.
- W3106239908 cites W2050268081 @default.
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- W3106239908 cites W2058468006 @default.
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- W3106239908 cites W2062597826 @default.
- W3106239908 cites W2066289545 @default.
- W3106239908 cites W2067271856 @default.
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- W3106239908 cites W2078966213 @default.
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- W3106239908 cites W2094346955 @default.
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- W3106239908 doi "https://doi.org/10.1063/1.4973975" @default.
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