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- W3106673060 endingPage "4149" @default.
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- W3106673060 abstract "Abstract An efficient approach to the type III lepadin alkaloids (lepadins F and G) has been developed through a key Diels–Alder reaction, in which a novel ketolactone‐type dienophile with chiral diol unit is employed to generate the desirable all‐ cis ‐trisubstituted cyclohexene with excellent regio‐ and stereoselectivity control. The subsequent selective sulfonylation of the diol unit followed by S N 2 cyclization under hydrogenation conditions could construct the substituted piperidine ring. By using this approach, (−)‐lepadin F is synthesized from ethyl l ‐lactate for the first time." @default.
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- W3106673060 date "2021-01-29" @default.
- W3106673060 modified "2023-09-24" @default.
- W3106673060 title "Total Synthesis of (−)‐Lepadin F based on a Stereoselective Diels–Alder Reaction Controlled by a Ketolactone‐type Dienophile" @default.
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- W3106673060 doi "https://doi.org/10.1002/chem.202004778" @default.
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