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• W3106945240 abstract "Abstract With their brilliance and temporal structure, X-ray free-electron laser can unveil atomic-scale details of ultrafast phenomena. Recent progress in split-and-delay optics (SDO), which produces two X-ray pulses with time-delays, offers bright prospects for observing dynamics at the atomic-scale. However, their insufficient pulse energy has limited its application either to phenomena with longer correlation length or to measurement with a fixed delay-time. Here we show that the combination of the SDO and self-seeding of X-rays increases the pulse energy and makes it possible to observe the atomic-scale dynamics in a timescale of picoseconds. We show that the speckle contrast in scattering from water depends on the delay-time as expected. Our results demonstrate the capability of measurement using the SDO with seeded X-rays for resolving the dynamics in temporal and spatial scales that are not accessible by other techniques, opening opportunities for studying the atomic-level dynamics." @default.
• W3106945240 created "2020-12-07" @default.
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• W3106945240 date "2020-12-04" @default.
• W3106945240 modified "2023-10-18" @default.
• W3106945240 title "Split-pulse X-ray photon correlation spectroscopy with seeded X-rays from X-ray laser to study atomic-level dynamics" @default.
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• W3106945240 doi "https://doi.org/10.1038/s41467-020-20036-z" @default.
• W3106945240 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7718898" @default.
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