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- W3107008484 abstract "Self-reporting fluorescence methods for monitoring folding and aggregation of proteins have a long history in biochemistry. Placing orthogonal luminophores within individual synthetic polymer chains for self-reporting both folding (i.e., its intramolecular compaction to isolated single-chain nanoparticles, SCNPs) and unbidden aggregation (i.e., the intermolecular association of SCNPs) remains a great challenge. Herein, a simple and efficient platform to identify both single-chain compaction and intermolecular aggregation phenomena via photoluminescence is presented based on simultaneous synthesis through Hantzsch ester formation of orthogonal luminophores within the same polymer chain. Starting from non-luminescent β-ketoester-decorated chains, intramolecular compaction is visually detected through fluorescence arising from Hantzsch fluorophores generated as intra-chain connectors during folding. Complementary, intermolecular association is identified via aggregation-induced emission (AIE) from orthogonal luminophores displaying intense photoluminescence at redshifted wavelengths after formation of multi-SCNPs assemblies." @default.
- W3107008484 created "2020-12-07" @default.
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- W3107008484 date "2020-12-14" @default.
- W3107008484 modified "2023-10-06" @default.
- W3107008484 title "Self‐Reporting of Folding and Aggregation by Orthogonal Hantzsch Luminophores Within a Single Polymer Chain" @default.
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- W3107008484 doi "https://doi.org/10.1002/anie.202013932" @default.
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