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- W3107402013 endingPage "781" @default.
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- W3107402013 abstract "Methanol, a versatile chemical, fuel additive and potential H2 carrier, has attracted great attention. Despite of the wide industrialization, improvement of Cu-based methanol-synthesis catalysts is highly anticipated. Accordingly, a series of Cu/ZnO/Al2O3 with designed precursor structures were prepared, and its structure–function relationship was investigated to make progress on this area. Results showed the catalyst derived from highly zinc-substituted malachite demonstrated the best catalytic performance in this work. It was found that the well-behaved catalyst possessed relatively high Cu specific surface area and exposed Cu concentration, and the well Cu/ZnO synergy. CuZn alloy was found by In-situ XRD tests, and its effect on the catalyst's thermostability was discussed. Fractional precipitation, which facilitated the Cu2+ substitution by Zn2+ in malachite lattice, could be an efficient preparation method of the Cu/ZnO/Al2O3 catalyst." @default.
- W3107402013 created "2020-12-07" @default.
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- W3107402013 date "2022-08-01" @default.
- W3107402013 modified "2023-10-15" @default.
- W3107402013 title "Improved methanol synthesis performance of Cu/ZnO/Al2O3 catalyst by controlling its precursor structure" @default.
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- W3107402013 doi "https://doi.org/10.1016/j.gee.2020.11.027" @default.
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