FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W3107530460> ?p ?o ?g. }

• W3107530460 endingPage "13" @default.
• W3107530460 startingPage "8" @default.
• W3107530460 abstract "Matrix-assisted ionization (MAI) demonstrates high sensitivity for a variety of organic compounds; however, few studies have reported the application of MAI for the detection and characterization of inorganic analytes. Trace-level uranium analysis is important in the realms of nuclear forensics, nuclear safeguards, and environmental monitoring. Traditional mass spectrometry methods employed in these fields require combinations of extensive laboratory chemistry sample preparation and destructive ionization methods. There has been recent interest in exploring ambient mass spectrometry methods that enable timely sample analysis and higher sensitivity than what is attainable by field-portable radiation detectors. Rapid characterization of uranium at nanogram levels is demonstrated in this study using MAI techniques. Mass spectra were collected on an atmospheric pressure mass spectrometer for solutions of uranyl nitrate, uranyl chloride, uranyl acetate, and uranyl oxalate utilizing 3-nibrobenzonitrile as the ionization matrix. The uranyl complexes investigated were detectable, and the chemical speciation was preserved. Sample analysis was accomplished in a matter of seconds, and limits of detection of 5 ng of uranyl nitrate, 10 ng of uranyl oxalate, 100 ng of uranyl chloride, and 200 ng of uranyl acetate were achieved. The observed gas-phase speciation was similar to negative-ion electrospray ionization of uranyl compounds with notable differences. Six matrix-derived ions were detected in all negative-ion mass spectra, and some of these ions formed adducts with the uranyl analyte. Subsequent analysis of the matrix suggests that these molecules are not matrix contaminants and are instead created during the ionization process." @default.
• W3107530460 created "2020-12-07" @default.
• W3107530460 creator A5029065709 @default.
• W3107530460 creator A5036542772 @default.
• W3107530460 creator A5060775683 @default.
• W3107530460 creator A5081315395 @default.
• W3107530460 date "2020-11-30" @default.
• W3107530460 modified "2023-09-26" @default.
• W3107530460 title "Matrix-Assisted Ionization of Molecular Uranium Species" @default.
• W3107530460 cites W1782817180 @default.
• W3107530460 cites W1968822050 @default.
• W3107530460 cites W1969890869 @default.
• W3107530460 cites W1971819072 @default.
• W3107530460 cites W1978009676 @default.
• W3107530460 cites W1978293365 @default.
• W3107530460 cites W1983728693 @default.
• W3107530460 cites W1984360801 @default.
• W3107530460 cites W1985310655 @default.
• W3107530460 cites W1989027151 @default.
• W3107530460 cites W1990321626 @default.
• W3107530460 cites W1994146016 @default.
• W3107530460 cites W2000337205 @default.
• W3107530460 cites W2002101949 @default.
• W3107530460 cites W2004511375 @default.
• W3107530460 cites W2005798334 @default.
• W3107530460 cites W2011166194 @default.
• W3107530460 cites W2017616870 @default.
• W3107530460 cites W2029058955 @default.
• W3107530460 cites W2037306155 @default.
• W3107530460 cites W2037470080 @default.
• W3107530460 cites W2041928276 @default.
• W3107530460 cites W2045328210 @default.
• W3107530460 cites W2047211427 @default.
• W3107530460 cites W2058150733 @default.
• W3107530460 cites W2073453473 @default.
• W3107530460 cites W2074088956 @default.
• W3107530460 cites W2091919232 @default.
• W3107530460 cites W2094423254 @default.
• W3107530460 cites W2104367814 @default.
• W3107530460 cites W2118376549 @default.
• W3107530460 cites W2136309037 @default.
• W3107530460 cites W2146268690 @default.
• W3107530460 cites W2247826386 @default.
• W3107530460 cites W2263049781 @default.
• W3107530460 cites W2290816085 @default.
• W3107530460 cites W2314895770 @default.
• W3107530460 cites W2331032609 @default.
• W3107530460 cites W2468557982 @default.
• W3107530460 cites W2470533244 @default.
• W3107530460 cites W2515115614 @default.
• W3107530460 cites W2528752521 @default.
• W3107530460 cites W2562582084 @default.
• W3107530460 cites W2735181135 @default.
• W3107530460 cites W2754410899 @default.
• W3107530460 cites W2779540988 @default.
• W3107530460 cites W2792765108 @default.
• W3107530460 cites W2807569170 @default.
• W3107530460 cites W2888101263 @default.
• W3107530460 cites W2888376683 @default.
• W3107530460 cites W2901663400 @default.
• W3107530460 cites W2909129587 @default.
• W3107530460 cites W2954593979 @default.
• W3107530460 cites W3007864445 @default.
• W3107530460 doi "https://doi.org/10.1021/jasms.0c00305" @default.
• W3107530460 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33253565" @default.
• W3107530460 hasPublicationYear "2020" @default.
• W3107530460 type Work @default.
• W3107530460 sameAs 3107530460 @default.
• W3107530460 citedByCount "2" @default.
• W3107530460 countsByYear W31075304602022 @default.
• W3107530460 countsByYear W31075304602023 @default.
• W3107530460 crossrefType "journal-article" @default.
• W3107530460 hasAuthorship W3107530460A5029065709 @default.
• W3107530460 hasAuthorship W3107530460A5036542772 @default.
• W3107530460 hasAuthorship W3107530460A5060775683 @default.
• W3107530460 hasAuthorship W3107530460A5081315395 @default.
• W3107530460 hasBestOaLocation W31075304602 @default.
• W3107530460 hasConcept C106487976 @default.
• W3107530460 hasConcept C113196181 @default.
• W3107530460 hasConcept C145148216 @default.
• W3107530460 hasConcept C162356407 @default.
• W3107530460 hasConcept C162633436 @default.
• W3107530460 hasConcept C178790620 @default.
• W3107530460 hasConcept C179104552 @default.
• W3107530460 hasConcept C185592680 @default.
• W3107530460 hasConcept C191897082 @default.
• W3107530460 hasConcept C192562407 @default.
• W3107530460 hasConcept C198291218 @default.
• W3107530460 hasConcept C205759337 @default.
• W3107530460 hasConcept C2776351790 @default.
• W3107530460 hasConcept C2776748962 @default.
• W3107530460 hasConcept C2778468930 @default.
• W3107530460 hasConcept C40684141 @default.
• W3107530460 hasConcept C43617362 @default.
• W3107530460 hasConcept C51884965 @default.
• W3107530460 hasConcept C555451288 @default.
• W3107530460 hasConceptScore W3107530460C106487976 @default.
• W3107530460 hasConceptScore W3107530460C113196181 @default.

• next