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• W3107677358 abstract "Titanium electrodes coated with transition metal oxides are used in many applications such as the electrogeneration of hydroxyl radicals ( • OH) via catalytic water oxidation. Here, we present electrochemical measurements of IrO 2 -Ta 2 O 5 |Ti electrodes with four different Ir:Ta ratios in the coating (100:0, 70:30, 30:70, 0:100) to better understand their electrochemical behavior. From the results, an Ir:Ta content of 70:30 reveals a homogeneous morphology, an outstanding mechanical stability, and the best generation of • OH radicals due to a cooperative enhancement of the electrocatalytic and proton (H + ) transfer properties of IrO 2 and Ta 2 O 5 , which are complemented by a small ohmic drop due to a junction established during the electrophoretic deposition of IrO 2 and Ta 2 O 5 . The electrochemical data in this work in conjunction with density functional theory calculations provide in-depth insights into the outstanding electrocatalytic properties of the as-prepared IrO 2 -Ta 2 O 5 |Ti electrodes, which may have applications in environmental processes. • IrO 2 -Ta 2 O 5 |Ti electrodes were constructed by electrophoretic deposition. • IrO 2 -Ta 2 O 5 |Ti electrodes with four different Ir:Ta ratios were prepared. • Ir:Ta (70:30) reveals a homogeneous morphology and mechanical stability. • Ir:Ta (70:30) has the best • OH radical generation performance as well as a long lifetime. • DFT calculations were applied to comprehend on the electrocatalytic properties of the as-prepared IrO 2 -Ta 2 O 5 |Ti electrodes." @default.
• W3107677358 created "2020-12-07" @default.
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• W3107677358 date "2021-05-01" @default.
• W3107677358 modified "2023-10-12" @default.
• W3107677358 title "Characterization of Ti electrodes electrophoretically coated with IrO2-Ta2O5 films with different Ir:Ta molar ratios" @default.
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• W3107677358 doi "https://doi.org/10.1016/j.jallcom.2020.158015" @default.
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