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- W3107741379 abstract "Bismuth perovskites ABiO$_3$ (A = Sr, Ba) host a variety of peculiar phenomena including bond-disproportionated insulating phases and high-temperature superconductivity upon hole doping. While the mechanisms underlying these phenomena are still debated, off-diagonal electron-phonon ($e$-ph) coupling originating from the modulation of the orbital overlaps has emerged as a promising candidate. Here, we employ classical Monte Carlo simulations to study a semiclassical three-orbital model with off-diagonal $e$-ph interactions. We demonstrate the existence of a (bi)polaron correlations that persists in the model at high temperatures and for hole doping away from the bond-disproportionated insulating phase. Using a spatiotemporal regression analysis between various local quantities and the lattice degrees of freedom, we also identify the similarity between heating- and doping-induced melting of a bond-disproportionated insulator at a microscopic level. Our results imply that (bi)polaron physics can be a unifying concept that helps us understand the rich bismuth perovskite phase diagram." @default.
- W3107741379 created "2020-12-07" @default.
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- W3107741379 date "2021-03-16" @default.
- W3107741379 modified "2023-09-23" @default.
- W3107741379 title "Polaron and bipolaron tendencies in a semiclassical model for hole-doped bismuthates" @default.
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- W3107741379 doi "https://doi.org/10.1103/physrevb.103.115129" @default.
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