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- W3108563830 abstract "Green synthesis of adipic acid from renewable biomass is a very attractive goal of sustainable chemistry. Herein, we report efficient catalysts for a two-step transformation of cellulose-derived glucose into adipic acid via glucaric acid. Carbon nanotube-supported platinum nanoparticles are found to work efficiently for the oxidation of glucose to glucaric acid. An activated carbon-supported bifunctional catalyst composed of rhenium oxide and palladium is discovered to be powerful for the removal of four hydroxyl groups in glucaric acid, affording adipic acid with a 99 % yield. Rhenium oxide functions for the deoxygenation but is less efficient for four hydroxyl group removal. The co-presence of palladium not only catalyzes the hydrogenation of olefin intermediates but also synergistically facilitates the deoxygenation. This work presents a green route for adipic acid synthesis and offers a bifunctional-catalysis strategy for efficient deoxygenation." @default.
- W3108563830 created "2020-12-07" @default.
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- W3108563830 date "2021-01-14" @default.
- W3108563830 modified "2023-09-30" @default.
- W3108563830 title "Efficient Catalysts for the Green Synthesis of Adipic Acid from Biomass" @default.
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- W3108563830 doi "https://doi.org/10.1002/anie.202013843" @default.
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