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- W3108968085 abstract "A Pd-catalyzed asymmetric [5 + 2] cycloaddition reaction was developed for the synthesis of N-fused 1,3-oxazepines using vinylethylene carbonates and sulfamate-derived cyclic imines. Under mild reaction conditions, a series of optically active N-fused 1,3-oxazepines were synthesized in good yields (up to 89%) and enantioselectivities (up to 90 : 10 er), indicating this method as a straightforward approach to enantiomerically enriched 1,3-oxazepine derivatives. The synthetic utility of the presented reaction was further demonstrated by the successful transformation of the resulting 1,3-oxazepines to useful polycyclic N-fused 1,3-oxazepanes." @default.
- W3108968085 created "2020-12-07" @default.
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- W3108968085 date "2020-01-01" @default.
- W3108968085 modified "2023-10-15" @default.
- W3108968085 title "Pd-Catalyzed asymmetric [5 + 2] cycloaddition of vinylethylene carbonates and cyclic imines: access to <i>N</i>-fused 1,3-oxazepines" @default.
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- W3108968085 doi "https://doi.org/10.1039/d0ob02159h" @default.
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