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• W3109452144 endingPage "127978" @default.
• W3109452144 startingPage "127978" @default.
• W3109452144 abstract "A desire for renewable alternatives to fossil fuels can be achieved by utilizing CO2, H2O, and solar energy to generate solar fuels. A novel N-doped graphene oxide enfolded reduced titania (NGO-RT) composite was demonstrated for photocatalytic CO2 reduction into CH4. Later, a small amount of Pt NPs was deposited on NGO-RT that increases the catalytic performance towards CH4 formation. The optimized Pt1.0%-NGO-RT catalyst displayed a selective visible-light CO2 reduction into CH4 using a flow reactor system with ≈12 and ≈2 times higher activity than pristine RT and NGO-RT, respectively. The catalyst demonstrated long-term stability over 35 h. The photo-induced CO2 reduction mechanism was first validated through the electron transfer process, where charge trapping by Ti3+ states near the conduction band of RT plays a vital role in the selective CH4 evolution. These trapped electrons transfer from RT to the closely connected interface of N-doped graphene oxide and Pt NPs to restrict the recombination of electron/hole pair. The improved catalytic performance can be attributed to RT’s downward band bending at the NGO-RT interface, where electron transfer from RT to NGO decreases the charge recombination." @default.
• W3109452144 created "2020-12-07" @default.
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• W3109452144 date "2021-07-01" @default.
• W3109452144 modified "2023-09-30" @default.
• W3109452144 title "A novel N-doped graphene oxide enfolded reduced titania for highly stable and selective gas-phase photocatalytic CO2 reduction into CH4: An in-depth study on the interfacial charge transfer mechanism" @default.
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• W3109452144 doi "https://doi.org/10.1016/j.cej.2020.127978" @default.
• W3109452144 hasPublicationYear "2021" @default.
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