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- W3109478850 endingPage "110890" @default.
- W3109478850 startingPage "110890" @default.
- W3109478850 abstract "Activated CO2 adsorption sites are crucial for improving selectivity in photocatalytic CO2 reduction. Co-catalysts incorporating rare or noble metals have previously been required to achieve high CO2 selectivity (SCO2); thus, noble-metal-free catalysts with high SCO2 are desirable but challenging to realize. We introduced S-scheme heterojunction using noble-metal-free TiO2/MoS2/graphitic carbon nitride (g-C3N4) with a strong redox ability showing SCO2 > 90%. This heterostructure improved CO2 conversion, to levels 3.1 times higher than that of the g-C3N4 alone and exhibited sufficient kinetic overpotential (0.18 eV) to produce significant amounts of CH4. When the proportion of g-C3N4 was optimized, the specified TiO2/MoS2/g-C3N4 achieved high SCO2 (~90%) due to its improved CO2 adsorption, in turn due to the improved specific surface area and pore size distribution attributable to amino (−NH2) groups of g-C3N4. We introduced, a novel, noble-metal-free TiO2/MoS2/g-C3N4 heterostructure that maximizes the number of CO2 adsorption sites and charge carriers separation through interconnected components, and thus increases SCO2." @default.
- W3109478850 created "2020-12-07" @default.
- W3109478850 creator A5021790990 @default.
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- W3109478850 date "2021-03-01" @default.
- W3109478850 modified "2023-10-17" @default.
- W3109478850 title "CO2 selectivity of flower-like MoS2 grown on TiO2 nanofibers coated with acetic acid-treated graphitic carbon nitride" @default.
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- W3109478850 doi "https://doi.org/10.1016/j.solmat.2020.110890" @default.
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