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- W3109559743 abstract "Abstract In this work we present the solution‐synthesis of pyridine analogues to hexa‐ peri ‐hexabenzocoronene (HBC)—which might be called superpyridines—via a novel precursor design. The key step in our strategy was the pre‐formation of the C−C bonds between the 3/3’ positions of the pyridine and the adjacent phenyl rings—bonds that are otherwise unreactive and difficult to close under Scholl‐conditions. Apart from the synthesis of the parent compound we show that classical pyridine chemistry, namely oxidation, N ‐alkylation and metal‐coordination is applicable to the π‐extended analogue. Furthermore, we present basic physical chemical characterizations of the newly synthesized molecules. With this novel synthetic strategy, we hope to unlock the pyridine chemistry of nanographenes." @default.
- W3109559743 created "2020-12-07" @default.
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- W3109559743 date "2021-01-12" @default.
- W3109559743 modified "2023-09-30" @default.
- W3109559743 title "Pyridinic Nanographenes by Novel Precursor Design" @default.
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- W3109559743 doi "https://doi.org/10.1002/chem.202004983" @default.
- W3109559743 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7898602" @default.
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