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• W3109607221 abstract "Abstract High-intensity extreme ultraviolet (XUV) pulses from a free-electron laser can be used to create a nanoplasma in clusters. In reference Michiels et al (2020 Phys. Chem. Chem. Phys. 22 7828–34) we investigated the formation of excited states in an XUV-induced nanoplasma in ammonia clusters. In the present article we expand our previous study with a detailed analysis of the nanoplasma evolution and ion kinetics. We use a time-delayed UV laser as probe to ionize excited states of H and <?CDATA ${mathrm{H}}_{2}^{+}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline overflow=scroll> <mml:msubsup> <mml:mrow> <mml:mi mathvariant=normal>H</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>2</mml:mn> </mml:mrow> <mml:mrow> <mml:mo>+</mml:mo> </mml:mrow> </mml:msubsup> </mml:math> in the XUV-induced plasma. Employing covariance mapping techniques, we show that the correlated emission of protons plays an important role in the plasma dynamics. The time-dependent kinetic energy of the ions created by the probe laser is measured, revealing the charge neutralization of the cluster happens on a sub-picosecond timescale. Furthermore, we observe ro-vibrationally excited molecular hydrogen ions <?CDATA ${mathrm{H}}_{2}^{+{ast}}$?> <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline overflow=scroll> <mml:msubsup> <mml:mrow> <mml:mi mathvariant=normal>H</mml:mi> </mml:mrow> <mml:mrow> <mml:mn>2</mml:mn> </mml:mrow> <mml:mrow> <mml:mo>+</mml:mo> <mml:mo>*</mml:mo> </mml:mrow> </mml:msubsup> </mml:math> being ejected from the clusters. We rationalize our data through a qualitative model of a finite-size non-thermal plasma." @default.
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• W3109607221 date "2021-01-18" @default.
• W3109607221 modified "2023-09-25" @default.
• W3109607221 title "Evolution and ion kinetics of a XUV-induced nanoplasma in ammonia clusters" @default.
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• W3109607221 doi "https://doi.org/10.1088/1361-6455/abcf80" @default.
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