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- W3109678639 endingPage "116252" @default.
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- W3109678639 abstract "In this study, boron doped diamond (BDD) is utilized as a redox flow battery (RFB) electrode, demonstrating its capability with several low-cost redox couples for the first time. Active species cost, electrode corrosion, energy density, and power density are the current issues hindering the widespread adoption of RFBs. Several high-potential and low-cost redox couples, including Ce3+/Ce4+ and Mn2+/Mn3+, are shown to exhibit low overpotentials, high efficiency, and good cyclability on BDD electrodes. Using the Ce3+/Ce4+ redox couple, a formal potential of 1.67 V vs. SHE and a peak separation of 288 mV during cyclic voltammetry was obtained. Low-cost redox species significantly decrease RFB system cost while high potentials increase energy and power density. Demonstrated here, high potentials cannot be supported by traditional carbon-based RFB electrodes due to significant corrosion and gas evolution; however, the inherent properties of BDD negate this effect. This study exhibits the potential of BDD, as an alternative to traditional carbon-based electrodes, to enable a long cycle life, at high coulombic efficiencies, and with high-potential and low-cost redox couples." @default.
- W3109678639 created "2020-12-07" @default.
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- W3109678639 date "2021-01-01" @default.
- W3109678639 modified "2023-10-18" @default.
- W3109678639 title "Earth-abundant redox couples using durable boron doped diamond electrodes: Beyond vanadium redox couples" @default.
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- W3109678639 doi "https://doi.org/10.1016/j.apenergy.2020.116252" @default.
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