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• W3110147863 endingPage "107503" @default.
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• W3110147863 abstract "We systematically investigate the magnetic properties of Cu 4 – x Zn x (OH) 6 FBr using the neutron diffraction and muon spin rotation and relaxation ( μ SR) techniques. Neutron-diffraction measurements suggest that the long-range magnetic order and the orthorhombic nuclear structure in the x = 0 sample can persist up to x = 0.23 and 0.43, respectively. The temperature dependence of the zero-field μ SR spectra provides two characteristic temperatures, T A 0 and T λ , which are associated with the initial drop close to zero time and the long-time exponential decay of the muon relaxation, respectively. Comparison between T A 0 and T M from previously reported magnetic-susceptibility measurements suggest that the former comes from the short-range interlayer-spin clusters that persist up to x = 0.82. On the other hand, the doping level where T λ becomes zero is about 0.66, which is much higher than threshold of the long-range order, i.e., ∼0.4. Our results suggest that the change in the nuclear structure may alter the spin dynamics of the kagome layers and a gapped quantum-spin-liquid state may exist above x = 0.66 with the perfect kagome planes." @default.
• W3110147863 created "2020-12-07" @default.
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• W3110147863 date "2020-10-01" @default.
• W3110147863 modified "2023-10-17" @default.
• W3110147863 title "Magnetic Phase Diagram of Cu_4–xZn_x(OH)₆FBr Studied by Neutron-Diffraction and μSR Techniques*" @default.
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• W3110147863 doi "https://doi.org/10.1088/0256-307x/37/10/107503" @default.
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