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- W3112311830 abstract "A carbohydrate-based fullerene derivative (AcMal7-C61) is designed, synthesized and applied to a lamellar-forming high-χ block copolymer system, poly(3-hexylthiophene)-block-peracetylated maltoheptaose (P3HT-b-AcMal7), to actualize an ordered donor/acceptor (D/A) network. A well-defined D/A lamellar structure of the P3HT-b-AcMal7:AcMal7-C61 blend with sub-10 nm domain features is achieved upon thermal annealing. The AcMal7-C61 molecules are localized in the phase-separated AcMal7 nanodomains without causing the formation of fullerene crystals while maintaining the lamellar morphology up to 1:0.5 (D:A) blending ratio. The cross-sectional TEM observation and GISAXS measurement reveals that the P3HT-b-AcMal7 tends to spontaneously organize into lamellar structures oriented perpendicular to the film surface at the air/film interface while the domain orientation at the bottom interface depends on the nature of the substrate." @default.
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- W3112311830 date "2021-03-01" @default.
- W3112311830 modified "2023-10-13" @default.
- W3112311830 title "Carbohydrate-attached fullerene derivative for selective localization in ordered carbohydrate-block-poly(3-hexylthiophene) nanodomains" @default.
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- W3112311830 doi "https://doi.org/10.1016/j.carbpol.2020.117528" @default.
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