FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W3112705374> ?p ?o ?g. }

• W3112705374 abstract "Manipulating the strain effect of Ag without any foreign metals to boost its intrinsic oxygen reduction reaction (ORR) activity is intriguing, but it remains a challenge. Herein, we developed a class of Ag-based electrocatalysts with tunable strain structures for efficient ORR via ligand-assisted competitive decomposition of Ag-organic complexes (AgOCs). Benefiting from the superior coordination capability, 4,4'-bipyridine as a ligand triggered a stronger competition with NaBH4 for Ag ions during reduction-induced decomposition of AgOCs in comparison with the counterparts of the pyrazine ligand and the NO3- anion, which moderately modulated the compressive strain structure to upshift the d-band center of the catalyst and increase the electron density of Ag. Accordingly, the O2 adsorption was obviously improved, and the stronger repulsion effect between the Ag sites and the 4e ORR product, i.e., the electron-rich OH-, was generated to promote the desorption of OH- via the Ag-OH bond cleavage, which enabled more Ag sites to be regenerated after ORR. Both of these led to an enhancement to the intrinsic ORR activity of the Ag-based catalyst. This competitive decomposition of metal-organic complex strategy would provide a facile method to design other catalysts with the well-tuned strain structures for energy conversion and heterocatalysis." @default.
• W3112705374 created "2020-12-21" @default.
• W3112705374 creator A5019625216 @default.
• W3112705374 creator A5038314144 @default.
• W3112705374 creator A5063176529 @default.
• W3112705374 creator A5063777885 @default.
• W3112705374 creator A5073722575 @default.
• W3112705374 creator A5090105972 @default.
• W3112705374 date "2020-12-10" @default.
• W3112705374 modified "2023-09-24" @default.
• W3112705374 title "Boosting Oxygen Electroreduction over Strained Silver" @default.
• W3112705374 cites W1587396183 @default.
• W3112705374 cites W1915333672 @default.
• W3112705374 cites W1975256305 @default.
• W3112705374 cites W1978678929 @default.
• W3112705374 cites W1990019902 @default.
• W3112705374 cites W1994884307 @default.
• W3112705374 cites W2017809059 @default.
• W3112705374 cites W2040938447 @default.
• W3112705374 cites W2042509191 @default.
• W3112705374 cites W2045834077 @default.
• W3112705374 cites W2073358933 @default.
• W3112705374 cites W2075543957 @default.
• W3112705374 cites W2091661097 @default.
• W3112705374 cites W2093729282 @default.
• W3112705374 cites W2103364873 @default.
• W3112705374 cites W2160351044 @default.
• W3112705374 cites W2167035995 @default.
• W3112705374 cites W2298245557 @default.
• W3112705374 cites W2321991700 @default.
• W3112705374 cites W2515875760 @default.
• W3112705374 cites W2521003546 @default.
• W3112705374 cites W2522850096 @default.
• W3112705374 cites W2543301362 @default.
• W3112705374 cites W2731927301 @default.
• W3112705374 cites W2744776017 @default.
• W3112705374 cites W2755768317 @default.
• W3112705374 cites W2760442154 @default.
• W3112705374 cites W2783140628 @default.
• W3112705374 cites W2785792227 @default.
• W3112705374 cites W2801067763 @default.
• W3112705374 cites W2801801868 @default.
• W3112705374 cites W2891183178 @default.
• W3112705374 cites W2893229243 @default.
• W3112705374 cites W2893983022 @default.
• W3112705374 cites W2894341893 @default.
• W3112705374 cites W2906069767 @default.
• W3112705374 cites W2908931700 @default.
• W3112705374 cites W2921449599 @default.
• W3112705374 cites W2934313054 @default.
• W3112705374 cites W2945789685 @default.
• W3112705374 cites W2946549703 @default.
• W3112705374 cites W2953273084 @default.
• W3112705374 cites W3023124676 @default.
• W3112705374 cites W4239505891 @default.
• W3112705374 doi "https://doi.org/10.1021/acsami.0c17973" @default.
• W3112705374 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33300776" @default.
• W3112705374 hasPublicationYear "2020" @default.
• W3112705374 type Work @default.
• W3112705374 sameAs 3112705374 @default.
• W3112705374 citedByCount "2" @default.
• W3112705374 countsByYear W31127053742021 @default.
• W3112705374 countsByYear W31127053742023 @default.
• W3112705374 crossrefType "journal-article" @default.
• W3112705374 hasAuthorship W3112705374A5019625216 @default.
• W3112705374 hasAuthorship W3112705374A5038314144 @default.
• W3112705374 hasAuthorship W3112705374A5063176529 @default.
• W3112705374 hasAuthorship W3112705374A5063777885 @default.
• W3112705374 hasAuthorship W3112705374A5073722575 @default.
• W3112705374 hasAuthorship W3112705374A5090105972 @default.
• W3112705374 hasConcept C102931765 @default.
• W3112705374 hasConcept C116569031 @default.
• W3112705374 hasConcept C124681953 @default.
• W3112705374 hasConcept C147789679 @default.
• W3112705374 hasConcept C150394285 @default.
• W3112705374 hasConcept C161790260 @default.
• W3112705374 hasConcept C162711632 @default.
• W3112705374 hasConcept C170493617 @default.
• W3112705374 hasConcept C178790620 @default.
• W3112705374 hasConcept C179104552 @default.
• W3112705374 hasConcept C185592680 @default.
• W3112705374 hasConcept C192562407 @default.
• W3112705374 hasConcept C2777765701 @default.
• W3112705374 hasConcept C55493867 @default.
• W3112705374 hasConcept C71240020 @default.
• W3112705374 hasConceptScore W3112705374C102931765 @default.
• W3112705374 hasConceptScore W3112705374C116569031 @default.
• W3112705374 hasConceptScore W3112705374C124681953 @default.
• W3112705374 hasConceptScore W3112705374C147789679 @default.
• W3112705374 hasConceptScore W3112705374C150394285 @default.
• W3112705374 hasConceptScore W3112705374C161790260 @default.
• W3112705374 hasConceptScore W3112705374C162711632 @default.
• W3112705374 hasConceptScore W3112705374C170493617 @default.
• W3112705374 hasConceptScore W3112705374C178790620 @default.
• W3112705374 hasConceptScore W3112705374C179104552 @default.
• W3112705374 hasConceptScore W3112705374C185592680 @default.
• W3112705374 hasConceptScore W3112705374C192562407 @default.
• W3112705374 hasConceptScore W3112705374C2777765701 @default.
• W3112705374 hasConceptScore W3112705374C55493867 @default.
• W3112705374 hasConceptScore W3112705374C71240020 @default.

• next