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- W3112753983 abstract "Abstract Solar-driven water splitting can store the abundant yet intermittent solar energy efficiently and produce hydrogen as a clean and sustainable energy carrier. A straightforward approach to light-driven water splitting is to apply self-supported particulate photocatalysts. However, efficient overall water splitting using single photocatalyst to date is limited to the UV range of light where high solar-to-hydrogen conversion efficiency is not expected according to the solar irradiance. An alternative approach to capturing sunlight is to efficiently construct a Z-scheme system based on the two-step photoexcitation of a hydrogen evolution photocatalyst and an oxygen evolution photocatalyst, both having narrow band gaps. The Z-scheme pathway is exceptionally useful because the device voltage is divided into several contributions, and thus, the band gap of the photocatalytic material does not have to straddle both the hydrogen and oxygen evolution potentials. Hence, narrow band gap semiconductors that are active only for proton reduction or water oxidation can be employed to split water using solar energy. In this review, we summarize the progress on the photocatalytic Z-scheme water splitting. We focus on the challenges of the Z-scheme system and summarize the design strategies to overcome the obstacles and limitations." @default.
- W3112753983 created "2020-12-21" @default.
- W3112753983 creator A5046225712 @default.
- W3112753983 creator A5052267876 @default.
- W3112753983 date "2021-01-01" @default.
- W3112753983 modified "2023-10-14" @default.
- W3112753983 title "Photocatalytic Z-scheme water splitting" @default.
- W3112753983 doi "https://doi.org/10.1016/b978-0-12-820072-8.00004-4" @default.
- W3112753983 hasPublicationYear "2021" @default.
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