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• W3113076808 endingPage "33185" @default.
• W3113076808 startingPage "33178" @default.
• W3113076808 abstract "This work is an attempt to develop bio-based eco-friendly poly(benzoxazine-co-urethane) [poly(U-co-CDL-aee)] materials using cardanol-based benzoxazines (CDL) and hexamethylene diisocyanate (HMDI) to check their self-healing ability and thermal properties. CDL monomers were synthesized using cardanol, amino ethoxyethanol (aee) or 3-aminopropanol (3-ap), and paraformaldehyde through the Mannich reaction. Later, CDL-aee or CDL-3-ap monomers were copolymerized with a urethane precursor (HMDI), followed by ring-opening polymerization through thermal curing. The thermal properties of poly(U-co-CDL) were evaluated by differential scanning calorimetry (DSC) and thermogravimetric analysis (TGA). The self-healing behavior of the bio-based poly(U-co-CDL) was checked by applying a mild external pressure. The results revealed that the developed poly(U-co-CDL) showed repeatable self-healing ability due to supramolecular hydrogen-bonding interactions. Further, the self-healing ability of poly(U-co-CDL) was studied using density functional theory (DFT). From the above results, the developed material with superior self-healing ability can be used in the form of self-healing coatings and composites for various applications with extended shelf-life and reliability." @default.
• W3113076808 created "2020-12-21" @default.
• W3113076808 creator A5005485268 @default.
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• W3113076808 date "2020-12-14" @default.
• W3113076808 modified "2023-10-06" @default.
• W3113076808 title "Eco-Friendly Sustainable Poly(benzoxazine-<i>co</i>-urethane) with Room-Temperature-Assisted Self-Healing Based on Supramolecular Interactions" @default.
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• W3113076808 doi "https://doi.org/10.1021/acsomega.0c04840" @default.
• W3113076808 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7774256" @default.
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• W3113076808 hasPublicationYear "2020" @default.
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