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• W3113292725 abstract "• The hexagonal structure for x ≤ 0.6 is evolved to orthorhombic one for x ≥ 0.7. • Increased Al substitution for In lowers the phase transition temperature. • The second-order phase transition is changed to the first-order-like one near x = 0.7. • The ΔS max and ΔT ad maximized at x = 0.8 by the hysteresis-free metamagnetic phase transition. • Mechanism explained by the greatly distorted lattice near the critical composition. By gradually substituting Al for In in Gd 2 In 1−x Al x (0.4 ≤ x ≤ 1) system, the hexagonal structure for Gd 2 In 1−x Al x ( x ≤ 0.6) is gradually evolved into orthorhombic one for x ≥ 0.7. The phase transition temperature is monotonously decreased. At the critical composition of x = 0.7, the second-order phase transformation in hexagonal Gd 2 In 1−x Al x ( x ≤ 0.6) is evolved into the first-order-like metamagnetic one without conventional hysteresis in orthorhombic Gd 2 In 1−x Al x ( x ≥ 0.7), leading into the enhanced magnetic entropy change and adiabatic temperature change. A lambda-like anomaly on the C p -T curves is also caused. Due to being close to the phase borderline separating hexagonal and orthorhombic structure, such enhanced magnetocaloric effect is considered to be from the greatly distorted lattice." @default.
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• W3113292725 date "2021-04-01" @default.
• W3113292725 modified "2023-09-23" @default.
• W3113292725 title "Enhanced magnetocaloric effects in Gd2In1−xAlx (0.4 ≤ x ≤ 1) system by the hysteresis-free metamagnetism" @default.
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• W3113292725 doi "https://doi.org/10.1016/j.jmmm.2020.167648" @default.
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