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• W3113295259 endingPage "124621" @default.
• W3113295259 startingPage "124621" @default.
• W3113295259 abstract "In this research, bismuth vanadate-doped graphite felt (GF-BiVO 4 ) was successfully prepared by sol–gel method, in which BiVO 4 owned superior electro-Fenton (EF) and solar-photo-electro-Fenton (SPEF) performance. Combined with the analysis by X-ray diffractometer (XRD), field emission transmission electron microscopy (FE-TEM), nitrogen adsorption–desorption isotherms and cyclic voltammetry (CV), the changes of electrodes were reflected in structure and physicochemical properties. The doping of monoclinic BiVO 4 endued GF with a higher surface area and more electro-active sites and better electrode activity in comparison to Raw-GF. Then, the GFs were used as cathodes to detect •OH concentration with coumarin (COU) as probe molecule and to evaluate photoelectric performance with ciprofloxacin (CIP) in photocatalysis, EF and SPEF processes. The results demonstrated that the concentration of •OH followed an order of SPEF > EF > photocatalysis, which was consistent with the removal rate of CIP (99.8%, 99.4% and 21.2%, respectively) on GF-BiVO 4 at 5 min. Further, five degradation pathways of CIP in SPEF system were proposed including the attack on piperazine ring, oxidation on cyclopropyl group, decarboxylation and hydroxyl radical addition, oxidation on benzene group and defluorination. The study provides insights into the enhancement of EF and SPEF performance and the degradation pathway of CIP in SPEF. • BiVO 4 prepared by the sol–gel was doped on graphite felt. • GF-BiVO 4 exhibited higher specific surface area, pore volume and active sites. • BiVO 4 strengthened GF’s generation ability of ·OH in SPEF and EF. • The destruction of piperazine and quinolone ring in SPEF was proposed." @default.
• W3113295259 created "2020-12-21" @default.
• W3113295259 creator A5001583756 @default.
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• W3113295259 date "2021-04-01" @default.
• W3113295259 modified "2023-10-16" @default.
• W3113295259 title "BiVO4 prepared by the sol–gel doped on graphite felt cathode for ciprofloxacin degradation and mechanism in solar-photo-electro-Fenton" @default.
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• W3113295259 doi "https://doi.org/10.1016/j.jhazmat.2020.124621" @default.
• W3113295259 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33383458" @default.
• W3113295259 hasPublicationYear "2021" @default.
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