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• W3114406722 endingPage "754" @default.
• W3114406722 startingPage "748" @default.
• W3114406722 abstract "Anti-CO poisoning ability is significant in formic acid oxidation in the fuel cell technique. Herein, PdNi alloy supported on N-doped graphene aerogel (PdNi/GA-N) was found to have catalytic ability toward formic acid electrooxidation over a wide potential range because of the improved anti-CO poisoning ability. This catalyst was fabricated by simple freeze-drying of mixture solution of graphene aerogel, polyvinylpyrrolidone, Pd2+ and Ni2+ and the subsequent thermal annealing reduction approach in the N2/H2 atmosphere. Pd–Ni alloy particles anchored over the folding N-doped graphene surface with a porous hierarchical architecture structure in the 3D directions. It showed the catalytic performance of its maximum mass activity of 836 mA mg−1 in a broad potential range (0.2–0.6 V) for formic acid oxidation. The CO stripping experiment demonstrated its largely improved anti-CO poisoning ability with the peak potential of 0.67 V, approximately 60 and 40 mV less compared to those of Pd/GA-N and Pd/C samples. The high anti-CO poisoning ability and strong electronic effect resulting from the interaction between the 3D GA-N support and the Pd–Ni alloy makes it a promising catalyst for application in direct formic acid fuel cells." @default.
• W3114406722 created "2021-01-05" @default.
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• W3114406722 date "2021-08-01" @default.
• W3114406722 modified "2023-10-16" @default.
• W3114406722 title "PdNi/N-doped graphene aerogel with over wide potential activity for formic acid electrooxidation" @default.
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• W3114406722 doi "https://doi.org/10.1016/j.jechem.2020.12.007" @default.
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