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- W3114962053 abstract "We report a TFC membrane with 2-D MOF nanosheets gutter layer, which exhibited outstanding H 2 separation performance and excellent stability. • An ultrathin microporous polymer TFC membrane was fabricated. • The 2-D MOF nanosheets acted as gutter layer. • The influence of the gutter layer for gas separation performance were discussed. • The 2-D MOF nanosheets gutter layer can reduce the gas transmission resistance. • The TFC membranes exhibited excellent stability and gas separation performance. The polymeric gutter layers of current thin film composite membranes (TFCMs) suffer from high gas diffusion resistance and fast performance deterioration. We designed a TFC membrane consisting of an ultrathin 2-D MOF nanosheets gutter layer and an ultrathin selective microporous polymer top layer via interfacial polymerization for H 2 separation. The 2-D MOF nanosheets gutter layer was shown to be thin and highly permeable with extremely low resistance for gas transport, thereby maximizing the gas permeance of the resulting composite membranes. The resulting TFCMs exhibited outstanding H 2 permeance (8.2 × 10 −7 mol m −2 s −1 Pa −1 ) with an ideal H 2 /CO 2 selectivity of 12.3–12.6. In addition, the TFCMs showed excellent long-term stability due to the rigidity and integrity of the 2-D MOF nanosheets. This study is expected to provide a new approach to design high performance TFCMs for H 2 separation." @default.
- W3114962053 created "2021-01-05" @default.
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- W3114962053 date "2021-04-01" @default.
- W3114962053 modified "2023-09-26" @default.
- W3114962053 title "A microporous polymer TFC membrane with 2-D MOF nanosheets gutter layer for efficient H2 separation" @default.
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- W3114962053 doi "https://doi.org/10.1016/j.seppur.2020.118283" @default.
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