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• W3115087478 abstract "We investigate the crystal structure, magnetic properties, and crystalline-electric field of tetragonal, $I4_1/amd$, NaCeO$_2$. In this compound, Ce$^{3+}$ ions form a tetragonally elongated diamond lattice coupled by antiferromagnetic interactions ($Theta_{CW} = -7.69$ K) that magnetically order below $T_N = 3.18$ K. The Ce$^{3+}$ $J = 5/2$ crystalline-electric field-split multiplet is studied via inelastic neutron scattering to parameterize a $J_{eff} = 1/2$ ground state doublet comprised of states possessing mixed $|m_z rangle$ character. Neutron powder diffraction data reveal the onset of $A$-type antiferromagnetism with $mu=0.57(2)$ $mu_B$ moments aligned along the $c$-axis. The magnetic structure is consistent with the expectations of a frustrated Heisenberg $J_1$-$J_2$ model on the elongated diamond lattice with effective exchange values $J_1 > 4 J_2$ and $J_1 > 0$." @default.
• W3115087478 created "2021-01-05" @default.
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• W3115087478 date "2021-01-19" @default.
• W3115087478 modified "2023-09-24" @default.
• W3115087478 title "Antiferromagnetism and crystalline electric field excitations in tetragonal <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML><mml:msub><mml:mi mathvariant=normal>NaCeO</mml:mi><mml:mn>2</mml:mn></mml:msub></mml:math>" @default.
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• W3115087478 doi "https://doi.org/10.1103/physrevb.103.024430" @default.
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