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• W3115442541 endingPage "124986" @default.
• W3115442541 startingPage "124986" @default.
• W3115442541 abstract "Oily sludge (OS) is a hazardous waste and pyrolysis is a promising technology to achieve energy recovery and non-hazardous disposal simultaneously. However, the distribution of hazardous elements, including N/S/Cl and heavy metals, in pyrolytic products possibly causes secondary pollution. This study conducted a systematic research on hazardous elements flow during OS pyrolysis under variant temperature. Results showed that N/S/Cl in OS were distributed 44.77–15.51 wt%, 83.29–80.22 wt%, and 78.59–73.41 wt% into the solid residues after pyrolysis, respectively. Elevating pyrolysis temperature facilitated more N/S/Cl flowing into pyrolytic oil and gas. The macromolecular N-/S-/Cl-containing compounds, including amides, amines, nitriles, sulfonates, chloroalkanes, etc., were widely distributed in pyrolytic oil and gas products. The micromolecular N-/S-/Cl-containing pollutants released between 200 and 400 °C included HCN, NH3, NOx, H2S, CH4S, CS2, SO2, and HCl, which originated from the decomposition of the amine N, organic sulfide and sulfone-S, and inorganic Cl, respectively. The main pollutants released at above 400 °C included NH3, HCN, NOx, CS2, and SO2, which were derived from the decomposition of heterocyclic N and inorganic pyritic-S and sulfate-S. Moreover, the solid residues intercepted more than 60.0 wt% of total heavy metals, which should be concerned in the future." @default.
• W3115442541 created "2021-01-05" @default.
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• W3115442541 date "2021-05-01" @default.
• W3115442541 modified "2023-10-13" @default.
• W3115442541 title "Hazardous elements flow during pyrolysis of oily sludge" @default.
• W3115442541 cites W1121695921 @default.
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• W3115442541 doi "https://doi.org/10.1016/j.jhazmat.2020.124986" @default.
• W3115442541 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33388449" @default.
• W3115442541 hasPublicationYear "2021" @default.
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