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- W3115997714 abstract "[Ca24Al28O64]4+·4(H−) (abbreviated as C12A7-H−) powder containing H− species was synthesized to modify NiW catalyst. The incorporation of C12A7-H− increases the reaction rate constants and turnover frequencies of NiW catalysts in hydrodesulfurization (HDS) of dibenzothiophene (DBT). The characterization results show that the introduction of C12A7-H− promotes the reducibility of NiW catalysts, resulting in higher sulfidation degree and more Ni-W-S species. In spite of the fact that rim/edge sites ratios and Lewis acid sites are decreased, the introduction of C12A7-H− still increases the hydrogenation/direct desulfurization ratios of NiW catalysts in HDS of DBT. Furthermore, higher HDS rates of C12A7-H− modified NiW catalysts are also observed in HDS of 4,6-dimethyldibenzothiophene. These can be attributed to C12A7-H− material that may transfer active H species to NiW catalysts and thereby promote the hydrogenation selectivity of NiW catalyst." @default.
- W3115997714 created "2021-01-05" @default.
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- W3115997714 date "2021-04-01" @default.
- W3115997714 modified "2023-09-27" @default.
- W3115997714 title "NiW catalyst modified with C12A7-H− and its promotion to hydrogenation selectivity of hydrodesulfurization" @default.
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- W3115997714 doi "https://doi.org/10.1016/j.fuel.2020.120037" @default.
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