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- W3116811495 abstract "It is highly desirable to realize high-energy-density lithium-ion batteries consisting of nickel-rich layered oxide cathodes (Ni-rich NMC) and Si-based anodes. A critical challenge for Ni-rich NMC is its fast capacity degradation. In addition, the low initial Coulombic efficiency of the Si-based anode consumes the electrochemically active lithium from the cathode and decreases the energy density of full batteries considerably. We consider cathode and anode as a whole to simultaneously resolve the issues of both sides. Ni-rich LiNi0.65Mn0.20Co0.15O2 (LR-Ni65) consisting of a lithium-enriched gradient interphase layer (∼20 nm) is designed to supply excess electrochemically active lithium to compensate lithium loss at the anode and enhance cycling stability through regulating Li/Ni disorder in the cathode structure. We show that a LR-Ni65||Si/graphite pouch cell displays a capacity (3.29 Ah) greater than that for the counterpart using pristine Ni-rich NMC (2.95 Ah), as well as enhanced cycling stability with 88% capacity retention. The good compatibility with current Ni-rich NMC processing and facile synthesis make the as-fabricated cathode material promising for practical commercial application." @default.
- W3116811495 created "2021-01-05" @default.
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- W3116811495 date "2020-12-31" @default.
- W3116811495 modified "2023-10-14" @default.
- W3116811495 title "Prelithiated Li-Enriched Gradient Interphase toward Practical High-Energy NMC–Silicon Full Cell" @default.
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- W3116811495 doi "https://doi.org/10.1021/acsenergylett.0c02487" @default.
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