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• W3116973775 abstract "The detailed understanding and control of ionic transport pathways in the electrode/electrolyte interface is vital for realizing micro-scale energy storage devices and formulating adequate design principles. A planar device geometry with nanostructured thin solid polymer electrolyte (SPE) and potassium hydroxide (KOH) incorporated poly(N-vinyl imidazole) (PVI) is demonstrated for micro-supercapacitors (MSCs). The adsorption/desorption kinetics of ionic charges in the interfacial regime of ITO/PVI-KOH has been investigated for electrical double layer capacitance (EDLC) characteristics. A single-cell of ITO/PVI-KOH/ITO planar MSC shows the large variation in volumetric capacitance and capacitance retention characteristics when the thickness of PVI-KOH approaches the characteristic nanoscale. Moreover, ITO/PVI-KOH/ITO planar MSC consisting of five series-cells exhibits the maximum operating cell voltage of 5.0 V with maximum volumetric energy and power density of 0.056 mW h cm-3 and 6.89 mW cm-3, respectively. The electrochemical properties of planar MSC have been systematically studied so as to confirm how the anions and cations are separated at electrode/electrolyte interfaces by means of an electromotive force. Significantly, the hydrated PVI enables charge migration and separation of cations and anions at the electrode/electrolyte interfaces." @default.
• W3116973775 created "2021-01-05" @default.
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• W3116973775 date "2020-01-01" @default.
• W3116973775 modified "2023-09-26" @default.
• W3116973775 title "Ionic transport kinetics and enhanced energy storage in the electrode/poly(<i>N</i>-vinyl imidazole) interface for micro-supercapacitors" @default.
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• W3116973775 doi "https://doi.org/10.1039/d0ra08137j" @default.
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