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- W3117567984 abstract "Two-dimensional (2D) lead halide Ruddlesden–Popper perovskites (RPP) have recently emerged as a prospective material system for optoelectronic applications. Their self-assembled multi quantum-well structure gives rise to the novel interwell energy funnelling phenomenon, which is of broad interests for photovoltaics, light-emission applications, and emerging technologies (e.g., spintronics). Herein, we develop a realistic finite quantum-well superlattice model that corroborates the hypothesis of exciton delocalization across different quantum-wells in RPP. Such delocalization leads to a sub-50 fs coherent energy transfer between adjacent wells, with the efficiency depending on the RPP phase matching and the organic large cation barrier lengths. Our approach provides a coherent and comprehensive account for both steady-state and transient dynamical experimental results in RPPs. Importantly, these findings pave the way for a deeper understanding of these systems, as a cornerstone crucial for establishing material design rules to realize efficient RPP-based devices." @default.
- W3117567984 created "2021-01-05" @default.
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- W3117567984 date "2020-12-18" @default.
- W3117567984 modified "2023-10-16" @default.
- W3117567984 title "The Physics of Interlayer Exciton Delocalization in Ruddlesden–Popper Lead Halide Perovskites" @default.
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- W3117567984 doi "https://doi.org/10.1021/acs.nanolett.0c03800" @default.
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