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- W3118277210 abstract "Abstract Covalent organic frameworks (COFs) are promising materials for advanced molecular-separation membranes, but their wide nanometer-sized pores prevent selective gas separation through molecular sieving. Herein, we propose a MOF-in-COF concept for the confined growth of metal-organic framework (MOFs) inside a supported COF layer to prepare MOF-in-COF membranes. These membranes feature a unique MOF-in-COF micro/nanopore network, presumably due to the formation of MOFs as a pearl string-like chain of unit cells in the 1D channel of 2D COFs. The MOF-in-COF membranes exhibit an excellent hydrogen permeance (>3000 GPU) together with a significant enhancement of separation selectivity of hydrogen over other gases. The superior separation performance for H 2 /CO 2 and H 2 /CH 4 surpasses the Robeson upper bounds, benefiting from the synergy combining precise size sieving and fast molecular transport through the MOF-in-COF channels. The synthesis of different combinations of MOFs and COFs in robust MOF-in-COF membranes demonstrates the versatility of our design strategy." @default.
- W3118277210 created "2021-01-18" @default.
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- W3118277210 date "2021-01-04" @default.
- W3118277210 modified "2023-10-17" @default.
- W3118277210 title "MOF-in-COF molecular sieving membrane for selective hydrogen separation" @default.
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- W3118277210 doi "https://doi.org/10.1038/s41467-020-20298-7" @default.
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- W3118277210 hasPublicationYear "2021" @default.
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