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• W3118345352 startingPage "8446" @default.
• W3118345352 abstract "Abstract Hydrogen plays important roles in the on‐surface synthesis of carbon‐based materials in ultra‐high vacuum. The complex interplay between hydrogen and surface‐adsorbed polycyclic aromatic hydrocarbons (PAHs) is tracked by in situ time‐of‐flight secondary ion mass spectrometry (ToF‐SIMS) combined with isotope labeling. In situ deuterium labeling of prototypical PAHs, coronene (CR) and 7‐armchair graphene nanoribbons (GNRs), on Au(111) is achieved by annealing either in D 2 gas or in the vapor of perdeuterio‐acenaphthene. By following the mass spectra of in situ deuterated CR mixed with hydrogen‐CR, it is demonstrated that PAHs adsorbed at hot Au(111) surfaces continuously exchange hydrogen atoms. Also, D 2 present during the Ullmann coupling step leads to incorporation of deuterium and to shorter GNRs." @default.
• W3118345352 created "2021-01-18" @default.
• W3118345352 creator A5039774009 @default.
• W3118345352 date "2021-03-03" @default.
• W3118345352 modified "2023-10-18" @default.
• W3118345352 title "On‐Surface Hydrogen/Deuterium Isotope Exchange in Polycyclic Aromatic Hydrocarbons" @default.
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• W3118345352 doi "https://doi.org/10.1002/anie.202015552" @default.
• W3118345352 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33440054" @default.
• W3118345352 hasPublicationYear "2021" @default.
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