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- W3118952802 abstract "Self-assembled nanomaterials composed of amphiphilic oligomers with functional groups have been applied in the fields of biomimetic chemistry and on-demand delivery systems. Herein, we report the assembly behavior and unique properties of an emergent n-shaped rod–coil molecule containing an azobenzene (AZO) group upon application of an external stimulus (thermal, UV light). The n-shaped amphiphilic molecules comprising an aromatic segment based on anthracene, phenyl linked with azobenzene groups, and hydrophilic oligoether (chiral) segments self-assemble into large strip-like sheets and perforated-nanocage fragments in an aqueous environment, depending on the flexible oligoether chains. Interestingly, the nano-objects formed in aqueous solution undergo a morphological transition from sheets and nanocages to small one-dimensional nanofibers. These molecules exhibit reversible photo- and thermal-responsiveness, accompanied by a change in the supramolecular chirality caused by the conformational transitions of the rod backbone. The architecture of n-shaped amphiphilic molecules with a photosensitive group makes them ideal candidates for intelligent materials for applications in advanced materials science." @default.
- W3118952802 created "2021-01-18" @default.
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- W3118952802 date "2021-01-11" @default.
- W3118952802 modified "2023-10-15" @default.
- W3118952802 title "Stimuli-Responsive Supramolecular Chirality Switching and Nanoassembly Constructed by n-Shaped Amphiphilic Molecules in Aqueous Solution" @default.
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- W3118952802 doi "https://doi.org/10.1021/acs.langmuir.0c03190" @default.
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