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• W3119253065 abstract "Abstract Tetragonal garnet-type Li 7 La 3 Zr 2 O 12 is an important candidate solid electrolyte for all-solid-state lithium ion batteries because of its high ionic conductivity and large electrochemical potential window. Here we employ atomistic simulation methods to show that the most favourable disorder process in Li 7 La 3 Zr 2 O 12 involves loss of Li 2 O resulting in lithium and oxygen vacancies, which promote vacancy mediated self-diffusion. The activation energy for lithium migration (0.45 eV) is much lower than that for oxygen (1.65 eV). Furthermore, the oxygen migration activation energy reveals that the oxygen diffusion in this material can be facilitated at higher temperatures once oxygen vacancies form." @default.
• W3119253065 created "2021-01-18" @default.
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• W3119253065 date "2021-01-11" @default.
• W3119253065 modified "2023-09-26" @default.
• W3119253065 title "Self-diffusion in garnet-type Li7La3Zr2O12 solid electrolytes" @default.
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• W3119253065 doi "https://doi.org/10.1038/s41598-020-79919-2" @default.
• W3119253065 hasPubMedCentralId "https://www.ncbi.nlm.nih.gov/pmc/articles/7801511" @default.
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