Matches in SemOpenAlex for { <https://semopenalex.org/work/W3119461209> ?p ?o ?g. }
- W3119461209 endingPage "144522" @default.
- W3119461209 startingPage "144522" @default.
- W3119461209 abstract "Rising industrial interest in the application of nanomaterials for the remediation of contaminated sites has led to concern over the environmental fate of the nanoremediation agents used. A critical requirement in evaluating and understanding nanoparticle (NP) behaviour in porous media is the development of analytical methods capable of in situ monitoring of complex NP transport dynamics. Spectral induced polarization (SIP), a non-invasive geo-electrical technique, offers a promising tool for detecting and quantifying NPs in soil and aquifer media. However, its application for monitoring the spatial migration and attachment behaviour of NPs remains uninvestigated. Here, we present results from flow-through experiments where we monitored the transport of cobalt ferrite nanoparticles (CoFe-NPs) coated with Pluronic, an amphiphilic polymer, in natural aquifer sand columns. We coupled concentration breakthrough curve analysis with SIP monitoring and reactive transport modeling to relate spatiotemporal NP concentration distributions to geo-electrical signals. Changes in the real (σ′) conductivity at three different locations along the columns closely correlated with model-computed total (solid plus aqueous phase) NP concentrations during the propagation of a NP slug. The imaginary conductivity (σ″) correlated closely with the arrival of the NP-slug. However, during the receding front, bimodal σ″-signal peak behaviour was observed propagating through the columns, indicating the existence of complex in situ NP transport dynamics, potentially revealing the rupture of nanoclusters upon straining and their effect on bulk charge storage that may not be obvious from breakthrough curve data alone. Fitting of a double Cole-Cole relaxation model yielded distinct shifts in relaxation time (τ) associated with the polarization of smaller length-scale particles. Post-NP pulse τ and σ″ did not return to pre-injection values; these lingering signals were caused by retained NP concentrations as low as 8.8 mg kg−1. Our results support the applicability of SIP for spatial and temporal monitoring of NP distributions, with implications for the investigation of NP transport and nanoremediation strategies." @default.
- W3119461209 created "2021-01-18" @default.
- W3119461209 creator A5012016285 @default.
- W3119461209 creator A5037707164 @default.
- W3119461209 creator A5069945332 @default.
- W3119461209 creator A5070738531 @default.
- W3119461209 creator A5071817803 @default.
- W3119461209 date "2021-05-01" @default.
- W3119461209 modified "2023-10-14" @default.
- W3119461209 title "Spatiotemporal geo-electrical sensing of a Pluronic-coated cobalt ferrite nanoparticle slug in natural sand flow-through columns" @default.
- W3119461209 cites W1776447867 @default.
- W3119461209 cites W1970615227 @default.
- W3119461209 cites W1980043117 @default.
- W3119461209 cites W1998572303 @default.
- W3119461209 cites W2017835174 @default.
- W3119461209 cites W2026039351 @default.
- W3119461209 cites W2036195573 @default.
- W3119461209 cites W2036431518 @default.
- W3119461209 cites W2054693124 @default.
- W3119461209 cites W2068067174 @default.
- W3119461209 cites W2070266204 @default.
- W3119461209 cites W2081030079 @default.
- W3119461209 cites W2082700434 @default.
- W3119461209 cites W2095849807 @default.
- W3119461209 cites W2108025662 @default.
- W3119461209 cites W2111369104 @default.
- W3119461209 cites W2126171847 @default.
- W3119461209 cites W2262846667 @default.
- W3119461209 cites W2305928919 @default.
- W3119461209 cites W2314296404 @default.
- W3119461209 cites W2315953690 @default.
- W3119461209 cites W2331991113 @default.
- W3119461209 cites W2465785673 @default.
- W3119461209 cites W2564384436 @default.
- W3119461209 cites W2772795561 @default.
- W3119461209 cites W2783258834 @default.
- W3119461209 cites W2795074351 @default.
- W3119461209 cites W2896486838 @default.
- W3119461209 cites W2903561316 @default.
- W3119461209 cites W2936585715 @default.
- W3119461209 cites W2948304434 @default.
- W3119461209 cites W2965229772 @default.
- W3119461209 cites W2978325216 @default.
- W3119461209 cites W2999650090 @default.
- W3119461209 cites W3006104090 @default.
- W3119461209 cites W3015266392 @default.
- W3119461209 doi "https://doi.org/10.1016/j.scitotenv.2020.144522" @default.
- W3119461209 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/33486168" @default.
- W3119461209 hasPublicationYear "2021" @default.
- W3119461209 type Work @default.
- W3119461209 sameAs 3119461209 @default.
- W3119461209 citedByCount "5" @default.
- W3119461209 countsByYear W31194612092022 @default.
- W3119461209 countsByYear W31194612092023 @default.
- W3119461209 crossrefType "journal-article" @default.
- W3119461209 hasAuthorship W3119461209A5012016285 @default.
- W3119461209 hasAuthorship W3119461209A5037707164 @default.
- W3119461209 hasAuthorship W3119461209A5069945332 @default.
- W3119461209 hasAuthorship W3119461209A5070738531 @default.
- W3119461209 hasAuthorship W3119461209A5071817803 @default.
- W3119461209 hasConcept C105569014 @default.
- W3119461209 hasConcept C119599485 @default.
- W3119461209 hasConcept C127313418 @default.
- W3119461209 hasConcept C127413603 @default.
- W3119461209 hasConcept C138631740 @default.
- W3119461209 hasConcept C150394285 @default.
- W3119461209 hasConcept C155672457 @default.
- W3119461209 hasConcept C159985019 @default.
- W3119461209 hasConcept C171250308 @default.
- W3119461209 hasConcept C178790620 @default.
- W3119461209 hasConcept C185592680 @default.
- W3119461209 hasConcept C187320778 @default.
- W3119461209 hasConcept C191897082 @default.
- W3119461209 hasConcept C192562407 @default.
- W3119461209 hasConcept C42360764 @default.
- W3119461209 hasConcept C515602321 @default.
- W3119461209 hasConcept C58445606 @default.
- W3119461209 hasConcept C6648577 @default.
- W3119461209 hasConcept C69990965 @default.
- W3119461209 hasConcept C75622301 @default.
- W3119461209 hasConcept C76177295 @default.
- W3119461209 hasConceptScore W3119461209C105569014 @default.
- W3119461209 hasConceptScore W3119461209C119599485 @default.
- W3119461209 hasConceptScore W3119461209C127313418 @default.
- W3119461209 hasConceptScore W3119461209C127413603 @default.
- W3119461209 hasConceptScore W3119461209C138631740 @default.
- W3119461209 hasConceptScore W3119461209C150394285 @default.
- W3119461209 hasConceptScore W3119461209C155672457 @default.
- W3119461209 hasConceptScore W3119461209C159985019 @default.
- W3119461209 hasConceptScore W3119461209C171250308 @default.
- W3119461209 hasConceptScore W3119461209C178790620 @default.
- W3119461209 hasConceptScore W3119461209C185592680 @default.
- W3119461209 hasConceptScore W3119461209C187320778 @default.
- W3119461209 hasConceptScore W3119461209C191897082 @default.
- W3119461209 hasConceptScore W3119461209C192562407 @default.
- W3119461209 hasConceptScore W3119461209C42360764 @default.
- W3119461209 hasConceptScore W3119461209C515602321 @default.
- W3119461209 hasConceptScore W3119461209C58445606 @default.