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- W3119463072 abstract "Abstract Potassium-ion capacitors (KICs) are promising for sustainable and eco-friendly energy storage technologies, yet their slow reaction kinetics and poor cyclability induced by large K -ion size are a major obstacle toward practical applications. Herein, by employing black phosphorus nanosheets (BPNSs) as a typical high-capacity anode material, we report that BPNS anodes armored with an ultrathin oriented-grown metal–organic-framework (MOF) interphase layer (BPNS@MOF) exhibit regulated potassium storage behavior for high-performance KICs. The MOF interphase layers as protective layer with ordered pores and high chemical/mechanical stability facilitate K ion diffusion and accommodate the volume change of electrode, beneficial for improved reaction kinetics and enhanced cyclability, as evidenced by substantial characterizations, kinetics analysis and DFT calculations. Consequently, the BPNS@MOF electrode as KIC anodes exhibits outstanding cycle performance outperforming most of the reported state-of-art KICs so far." @default.
- W3119463072 created "2021-01-18" @default.
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- W3119463072 date "2021-01-04" @default.
- W3119463072 modified "2023-10-16" @default.
- W3119463072 title "Armoring Black Phosphorus Anode with Stable Metal–Organic-Framework Layer for Hybrid K-Ion Capacitors" @default.
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- W3119463072 doi "https://doi.org/10.1007/s40820-020-00570-7" @default.
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