Matches in SemOpenAlex for { <https://semopenalex.org/work/W3119645867> ?p ?o ?g. }
- W3119645867 endingPage "128419" @default.
- W3119645867 startingPage "128419" @default.
- W3119645867 abstract "The electro-catalytic nitrogen reduction reaction (NRR) to produce ammonia is a significant and challenging mission in chemistry, in which metal-free NRR catalysts with high activity, stability and selectivity are still highly desired. Here, we have systematically investigated the properties of pristine and carbon doped hexagonal boron nitride nanoribbons (BNNRs) for efficient nitrogen capture and reduction. Our results suggest that BNNRs exhibit excellent N2 capture abilities, which are demonstrated to be originated from the edge lone pair electrons. Then we highlight that doping carbon can significantly enhance the NRR catalytic performance of BNNRs by reducing the NRR reaction overpotential from 1.14 to 0.39 V. Further analysis unravels that doping C can selectively modulate the adsorption free energy of NRR intermediates without influencing the excellent activation ability of pristine BNNRs, which has been confirmed to arise from the charge redistribution of edge boron atoms. Our findings pave the way of h-BN for N2 capture and pioneer the application of carbon doped BNNR as a novel NRR catalyst." @default.
- W3119645867 created "2021-01-18" @default.
- W3119645867 creator A5003946857 @default.
- W3119645867 creator A5007682410 @default.
- W3119645867 creator A5022913125 @default.
- W3119645867 creator A5023704274 @default.
- W3119645867 creator A5024736552 @default.
- W3119645867 creator A5040401880 @default.
- W3119645867 creator A5047060524 @default.
- W3119645867 creator A5054091259 @default.
- W3119645867 creator A5060002817 @default.
- W3119645867 creator A5067318984 @default.
- W3119645867 creator A5069736534 @default.
- W3119645867 date "2021-04-01" @default.
- W3119645867 modified "2023-10-05" @default.
- W3119645867 title "Carbon doped hexagonal boron nitride nanoribbon as efficient metal-free electrochemical nitrogen reduction catalyst" @default.
- W3119645867 cites W1026426193 @default.
- W3119645867 cites W1618810017 @default.
- W3119645867 cites W1970127494 @default.
- W3119645867 cites W1971409718 @default.
- W3119645867 cites W1974324776 @default.
- W3119645867 cites W1976199200 @default.
- W3119645867 cites W1980072692 @default.
- W3119645867 cites W1981368803 @default.
- W3119645867 cites W1987730936 @default.
- W3119645867 cites W1999086537 @default.
- W3119645867 cites W2015294180 @default.
- W3119645867 cites W2026125534 @default.
- W3119645867 cites W2032421626 @default.
- W3119645867 cites W2045050011 @default.
- W3119645867 cites W2048110396 @default.
- W3119645867 cites W2051498249 @default.
- W3119645867 cites W2066414697 @default.
- W3119645867 cites W2072155013 @default.
- W3119645867 cites W2082276489 @default.
- W3119645867 cites W2091587267 @default.
- W3119645867 cites W2148707525 @default.
- W3119645867 cites W2156809317 @default.
- W3119645867 cites W2175951962 @default.
- W3119645867 cites W2414522883 @default.
- W3119645867 cites W2460396937 @default.
- W3119645867 cites W2460474067 @default.
- W3119645867 cites W2556334122 @default.
- W3119645867 cites W2744886316 @default.
- W3119645867 cites W2767966656 @default.
- W3119645867 cites W2781713722 @default.
- W3119645867 cites W2783848705 @default.
- W3119645867 cites W2788213189 @default.
- W3119645867 cites W2804705815 @default.
- W3119645867 cites W2808316403 @default.
- W3119645867 cites W2809808471 @default.
- W3119645867 cites W2848021223 @default.
- W3119645867 cites W2851584547 @default.
- W3119645867 cites W2888741751 @default.
- W3119645867 cites W2892230460 @default.
- W3119645867 cites W2904960620 @default.
- W3119645867 cites W2912813828 @default.
- W3119645867 cites W2913734789 @default.
- W3119645867 cites W2932830081 @default.
- W3119645867 cites W2936060683 @default.
- W3119645867 cites W2945651220 @default.
- W3119645867 cites W2947517642 @default.
- W3119645867 cites W2948018974 @default.
- W3119645867 cites W2964352157 @default.
- W3119645867 cites W2969888966 @default.
- W3119645867 cites W2983000192 @default.
- W3119645867 cites W3012129486 @default.
- W3119645867 cites W3042579480 @default.
- W3119645867 cites W3097598502 @default.
- W3119645867 cites W4246112865 @default.
- W3119645867 doi "https://doi.org/10.1016/j.cej.2021.128419" @default.
- W3119645867 hasPublicationYear "2021" @default.
- W3119645867 type Work @default.
- W3119645867 sameAs 3119645867 @default.
- W3119645867 citedByCount "49" @default.
- W3119645867 countsByYear W31196458672021 @default.
- W3119645867 countsByYear W31196458672022 @default.
- W3119645867 countsByYear W31196458672023 @default.
- W3119645867 crossrefType "journal-article" @default.
- W3119645867 hasAuthorship W3119645867A5003946857 @default.
- W3119645867 hasAuthorship W3119645867A5007682410 @default.
- W3119645867 hasAuthorship W3119645867A5022913125 @default.
- W3119645867 hasAuthorship W3119645867A5023704274 @default.
- W3119645867 hasAuthorship W3119645867A5024736552 @default.
- W3119645867 hasAuthorship W3119645867A5040401880 @default.
- W3119645867 hasAuthorship W3119645867A5047060524 @default.
- W3119645867 hasAuthorship W3119645867A5054091259 @default.
- W3119645867 hasAuthorship W3119645867A5060002817 @default.
- W3119645867 hasAuthorship W3119645867A5067318984 @default.
- W3119645867 hasAuthorship W3119645867A5069736534 @default.
- W3119645867 hasConcept C104779481 @default.
- W3119645867 hasConcept C127413603 @default.
- W3119645867 hasConcept C140205800 @default.
- W3119645867 hasConcept C147789679 @default.
- W3119645867 hasConcept C159985019 @default.
- W3119645867 hasConcept C161790260 @default.
- W3119645867 hasConcept C171250308 @default.
- W3119645867 hasConcept C17525397 @default.