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- W3119686516 abstract "Abstract Metal-organic layers with ordered structure and molecular tunability are of great potential as heterogeneous catalysts due to their readily accessible active sites. Herein, we demonstrate a facile template strategy to prepare metal-organic layers with a uniform thickness of three metal coordination layers (ca. 1.5 nm) with graphene oxide as both template and electron mediator. The resulting hybrid catalyst exhibits an excellent performance for CO 2 photoreduction with a total CO yield of 3133 mmol g –1 MOL (CO selectivity of 95%), ca. 34 times higher than that of bulky Co-based metal-organic framework. Systematic studies reveal that well-exposed active sites in metal-organic layers, and facile electron transfer between heterogeneous and homogeneous components mediated by graphene oxide, greatly contribute to its high activity. This work highlights a facile way for constructing ultrathin metal-organic layers and demonstrates charge transfer pathway between conductive template and catalyst for boosting photocatalysis." @default.
- W3119686516 created "2021-01-18" @default.
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- W3119686516 date "2021-02-05" @default.
- W3119686516 modified "2023-10-17" @default.
- W3119686516 title "Facile electron delivery from graphene template to ultrathin metal-organic layers for boosting CO2 photoreduction" @default.
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- W3119686516 doi "https://doi.org/10.1038/s41467-021-21084-9" @default.
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