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• W3119806398 endingPage "351" @default.
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• W3119806398 abstract "Bulk scintillators that are with high density, low cost, and fine pulse-height energy spectral resolution, and are non-hygroscopic and user friendly, are desired for high-energy gamma-ray spectroscopy application. Recently, low-cost solution-processed perovskite nanoscintillators have been demonstrated with outstanding performances for indirect low-energy X-ray detection; however, the stability and thickness are not suitable for high-energy gamma-ray detection. Here, we report scintillation performances of a low-cost solution-processed bulk 0D <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline id=m1> <mml:mrow> <mml:msub> <mml:mrow> <mml:mi>Cs</mml:mi> </mml:mrow> <mml:mn>3</mml:mn> </mml:msub> <mml:msub> <mml:mrow> <mml:mi>Cu</mml:mi> </mml:mrow> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi mathvariant=normal>I</mml:mi> <mml:mn>5</mml:mn> </mml:msub> </mml:mrow> </mml:math> single crystal. The self-trapped exciton emission results in a large Stokes shift (109 nm) that is reabsorption free. A broad X-ray excited emission matches well with the sensitivity of a silicon photodiode. The unique <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline id=m2> <mml:mrow> <mml:msup> <mml:mrow> <mml:mi>Cs</mml:mi> </mml:mrow> <mml:mo>+</mml:mo> </mml:msup> </mml:mrow> </mml:math> surrounded isolated <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline id=m3> <mml:mrow> <mml:msup> <mml:mrow> <mml:mo stretchy=false>[</mml:mo> <mml:msub> <mml:mrow> <mml:mi>Cu</mml:mi> </mml:mrow> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi mathvariant=normal>I</mml:mi> <mml:mn>5</mml:mn> </mml:msub> <mml:mo stretchy=false>]</mml:mo> </mml:mrow> <mml:mrow> <mml:mn>3</mml:mn> <mml:mo>−</mml:mo> </mml:mrow> </mml:msup> </mml:mrow> </mml:math> cluster scintillator provides ultra-stability in air and strong radiation hardness under high-dose gamma-ray exposure from a 60 Co source. This solution-processed <mml:math xmlns:mml=http://www.w3.org/1998/Math/MathML display=inline id=m4> <mml:mrow> <mml:msub> <mml:mrow> <mml:mi>Cs</mml:mi> </mml:mrow> <mml:mn>3</mml:mn> </mml:msub> <mml:msub> <mml:mrow> <mml:mi>Cu</mml:mi> </mml:mrow> <mml:mn>2</mml:mn> </mml:msub> <mml:msub> <mml:mi mathvariant=normal>I</mml:mi> <mml:mn>5</mml:mn> </mml:msub> </mml:mrow> </mml:math> scintillator is expected with low-cost and has detection performances comparable to commercial alkali-halide scintillator products." @default.
• W3119806398 created "2021-01-18" @default.
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• W3119806398 date "2021-02-22" @default.
• W3119806398 modified "2023-10-14" @default.
• W3119806398 title "Solution-processed lead-free bulk 0D Cs₃Cu₂I₅ single crystal for indirect gamma-ray spectroscopy application" @default.
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• W3119806398 doi "https://doi.org/10.1364/prj.412959" @default.
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